We study strong-field ionization by quantum lights with emphasis on high-order above-threshold ionization and the intensity-dependent enhancements in the photoelectron spectra. We find that the length of the plateau in the photoelectron energy spectrum generated by such quantum lights can be extended by an order of magnitude in comparison with that generated by the classical coherent laser light and that within this plateau resonantly enhanced groups of sharp peaks appear at energies which are integer multiple of the photon energy. We relate the observed intensity-dependent enhancements to the channel closing effect. Our results are particularly interesting in the context of the recent interplay and merging of quantum optics with strong-field physics and attoscience.

The complete classification of the saddle-point solutions for high-order above-threshold ionization, presented in and for a linearly polarized laser field, is generalized to the case of an arbitrary bichromatic elliptically polarized field. We first present the classification of the saddle-point solutions for the case of a monochromatic elliptically polarized driving field, which is the simplest example of the field that has two components, i.e., that evolves in the plane. For a bichromatic laser field whose elliptically polarized components have the frequencies rω and sω (r and s are integers, s>r, and ω is the fundamental frequency), the system of the saddle-point equations has 8s2 solutions per optical cycle. One-half of these solutions are the so-called backward-scattering solutions for which the direction of the electron motion is significantly affected by the rescattering. The other half are the forward-scattering solutions for which the electron is only slightly deflected during the rescattering event. For some specific field configurations, the number of saddle-point solutions can be smaller. For example, for a bicircular field, which consists of two counterrotating circularly polarized components, there are 4s(r+s) solutions, while for the corotating configuration there are 4s2 solutions. As an application, we have shown that for a monochromatic elliptically polarized laser field, all four threshold anomalies appear in the spectra of the rescattered photoelectrons.

For decades the strong-field approximation (SFA) has been a theoretical backbone for describing the strong-field related phenomena such as above-threshold ionization (ATI) and high-order harmonic generation, even though it is well-known that it cannot accurately account for the long-range Coulomb interaction between the liberated electron and residual atomic ion. In this paper, we theoretically investigate high-order ATI. We use numerical solutions of the time-dependent Schrödinger equation (TDSE) and an improved SFA that includes electron rescattering. The analysis is performed for atomic anions and neutral atoms exposed to elliptically polarized laser fields. To validate the SFA and test its applicability, we compare both theoretical approaches for various targets and laser field parameters. We also show that the improved SFA in which the final electron plane wave is replaced by the Coulomb distorted plane wave leads to a better agreement with the results obtained using the solutions of the TDSE.

When the strong-field ionization of atoms is induced by an ultrashort pulse instead of a long pulse with a flat envelope, many symmetry properties of the photoelecton momentum distribution are broken. The induced asymmetry is measured using the asymmetry parameter which depends on the values of the driving-pulse parameters and the type of the target. We investigate the driving pulses with two carrier frequencies because in this case the dependence of the asymmetry on the characteristics of the target is more robust. Particular attention is devoted to the pulse which consists of two circularly polarized few-cycle waves and the pulse which has two linearly polarized components with mutually orthogonal polarizations. In the former case, we show that the asymmetry parameter is highly sensitive to the ionization potential and to the structure of the ground state. This is particularly the case for the photoelectron energy just above the value for which the contribution of the electrons which do not interact with the core after the ionization becomes negligible. We explain this sensitivity by investigating the dependence of the short-travel-time saddle-point solutions on the characteristics of the target. On the other hand, for the driving pulse with linearly polarized components, the dependence of the asymmetry parameter on the ionization potential is significant, while the dependence on the structure of the ground state is relatively small. In conclusion, we show that the characteristics of the target are imprinted in the asymmetry parameter and this signature is more pronounced for two-component pulses than for the linearly polarized driving pulse with one carrier frequency. Published by the American Physical Society 2025

The saddle-point solutions for strong-laser-field-induced high-order above-threshold ionization, the complete classification of which was recently presented in , are considered classically. In the limit of vanishing ionization potential the system of saddle-point equations simplifies, allowing a semi-analytical treatment. For a monochromatic field, the analytical nonlinear equations obtained this way allow one to determine the maximum (cutoff) photoelectron energies for the backward- and forward-scattering saddle-point solutions for all values of the multi-indices introduced by our classification scheme. These cutoffs are determined for all photoelectron momenta and it is shown how the backward-scattering solutions from one half of the momentum plane are related to the forward-scattering solutions from the other. The case of a bichromatic linearly polarized field is analyzed in detail. The results are rederived with the help of a simple graphical method, which can be used to qualitatively discuss the effect of varying the field parameters. Published by the American Physical Society 2025

Above-threshold detachment of electrons from negative ions by a strong low-frequency elliptically polarized laser field is considered using the strong-field approximation. The detachment probability amplitude is expressed via integral over times of highly oscillatory functions. Particular attention is devoted to application of the asymptotic methods to solve these integrals. For the direct detachment only the integral over the detachment time appears, while for the high-order above-threshold detachment the double integral over the detachment and rescattering times should be solved. Depending on the ellipticity of the laser field, a critical photoelectron energy exists for which the standard saddle-point method fails. The problem can be solved by properly deforming the integration contour in the complex time plane and, for energies higher than this critical energy, taking into account only one of the two saddle-point solutions. However, this procedure still leaves a spike in the photoelectron spectrum near this critical energy. This problem is cured applying the uniform approximation. A formula for the transition amplitude in the uniform approximation is derived, and it is shown how this formula should be modified for the energies higher than the critical one. For high-order above-threshold detachment many more saddle-point solutions contribute. They are classified into pairs. For the saddle-point method each pair produces a spike in the spectrum which spoils the total spectrum. When the contribution of each pair is treated using the uniform approximation with a careful choice of the phase factors after the anti-Stokes transition the agreement with the exact numerical results becomes excellent. Published by the American Physical Society 2025

Ionization of atoms by a strong laser field can be described using the improved strong-field approximation. The corresponding transition amplitude of high-order above-threshold ionization is presented in the form of a two-dimensional integral over the electron ionization time t0 and the rescattering time t. This integral can be solved using the saddle-point (SP) method and the resulting T-matrix element is expressed as a sum (over the SP times t0 and t) of the partial transition amplitudes. We address the problem of finding the solutions of the system of SP equations for the times t0 and t. For a bichromatic linearly polarized laser field with the frequencies rω and sω (r and s are integers, s>r, and ω is the fundamental frequency) we found that there are 8s2 SP solutions per optical cycle. For one half of them the velocity of the electron emitted in the laser field polarization direction changes the sign at the rescattering time (we call such solutions backward-scattering solutions), while for the other half this velocity remains unchanged (these solutions we call forward-scattering SP solutions). For very short (or even negative) electron travel time we call these solutions backward-like and forward-like scattering SP solutions. For these solutions the imaginary parts of the times t0 and t become large so that the concept of real electron trajectories becomes questionable. Having such a classification, we found additional SP solutions even for the simplest case of a monochromatic linearly polarized laser field. For a bichromatic linearly polarized laser field with s=2 and equal component intensities we presented a detailed analysis of all 32 solutions per optical cycle, showing how the SP times t0 and t and the corresponding differential ionization rates depend on the photoelectron energy. We have also analyzed the case where the intensity of the second component decreases while the sum of the component intensities remains fixed. Published by the American Physical Society 2025

When nonsequential double ionization is treated using the strong-field approximation and the saddle-point (SP) method, the transition amplitude can be expressed as a coherent sum of the partial amplitudes corresponding to different SP solutions. For the case of the recollision excitation with subsequent ionization (RESI) mechanism of the nonsequential double ionization, we examine the partial contributions of the SP solutions which correspond to the electron responsible for the excitation. For a monochromatic linearly polarized laser field, we find that, in addition to the pair of the SP solutions with the shortest travel time, other SP solutions may also make a significant contribution to the photoelectron yield. Moreover, the SP solutions appear in pairs and exhibit notable modifications in comparison to those observed in high-order above-threshold ionization. Furthermore, for a bichromatic linearly polarized driving field, we investigate the intensity range obtained using the simpleman’s model for which the RESI mechanism is dominant. We find that this range must be modified if the photoelectron yield corresponding to the SP solution for which the photoelectron has the highest energy upon return to the parent ion is small. This is particularly the case for the excitation channels involving loosely bound excited states.